Title: Decomposition of atrazine traces in water by combination of non-thermal electrical discharge and adsorption on nanofiber membrane
Authors: Vanraes, Patrick ×
Willems, Gert
Daels, Nele
Van Hulle, Stijn
De Clerck, Karen
Lynen, Frederick
Vandamme, Jeroen
Van Durme, Jim
Nikiforov, Anton
Leys, Christophe #
Issue Date: 1-Apr-2015
Publisher: Pergamon Press
Series Title: Water Research vol:72 pages:361-371
Abstract: In recent decades, several types of persistent substances are detected in the aquatic environment at very low concentrations. Unfortunately, conventional water treatment processes are not able to remove these micropollutants. As such, advanced treatment methods are required to meet both current and anticipated maximally allowed concentrations. Plasma discharge in contact with water is a promising new technology, since it produces a wide spectrum of oxidizing species. In this study, a new type of reactor is tested, in which decomposition by atmospheric pulsed direct barrier discharge (pDBD) plasma is combined with micropollutant adsorption on a nanofiber polyamide membrane. Atrazine is chosen as model micropollutant with an initial concentration of 30 μg/L. While the H2O2 and O3 production in the reactor is not influenced by the presence of the membrane, there is a significant increase in atrazine decomposition when the membrane is added. With membrane, 85% atrazine removal can be obtained in comparison to only 61% removal without membrane, at the same experimental parameters. The by-products of atrazine decomposition identified by HPLC-MS are deethylatrazine and ammelide. Formation of these by-products is more pronounced when the membrane is added. These results indicate the synergetic effect of plasma discharge and pollutant adsorption, which is attractive for future applications of water treatment.
ISSN: 0043-1354
Publication status: published
KU Leuven publication type: IT
Appears in Collections:Bioengineering Technology TC, Technology Campuses Ghent and Aalst
Technologiecluster Bioengineering Technologie
× corresponding author
# (joint) last author

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