Title: The non-linear refractive index of colloidal PbSe nanocrystals: Spectroscopy and saturation behaviour
Authors: Moreels, I ×
Kockaert, P
Van Deun, Rik
Driesen, Kris
Loicq, J
Van Thourhout, D
Hens, Z #
Issue Date: Jan-2006
Publisher: Elsevier science bv
Series Title: Journal of luminescence vol:121 issue:2 pages:369-374
Abstract: A spectroscopic study of the optical non-linearities of PbSe colloidal solutions was performed with the Z-scan technique, at wavelengths between 1200 and 1750 nm. No non-linear absorption is observed, while the third-order non-linear refractive index it, shows clear resonances, somewhat blueshifted relative to the exciton transitions in the absorbance spectrum. The occurrence of thermal effects is ruled out by time-resolved measurements. At resonance, measured it, values exceed typical bulk semiconductor values by two orders of magnitude. At high optical intensity, the refractive index change saturates, indicating that state filling lies at the origin of the observed effect. (c) 2006 Elsevier B.V. All rights reserved.
ISSN: 0022-2313
Publication status: published
KU Leuven publication type: IT
Appears in Collections:Molecular Design and Synthesis
× corresponding author
# (joint) last author

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