Title: Conversion of carbon dioxide to value-added chemicals in atmospheric pressure dielectric barrier discharges
Authors: Paulussen, Sabine ×
Verheyde, Bert
Tu, Xin
De Bie, Christophe
Martens, Tom
Petrovic, Dragana
Bogaerts, Annemie
Sels, Bert #
Issue Date: Jun-2010
Publisher: IOP Pub.
Series Title: Plasma Sources Science & Technology vol:19 issue:3 pages:034015/1-034015/6
Conference: The 29th International Conference on Phenomena in Ionized Gases location:Cancún, Mexico date:12-17 July 200
Abstract: The aim of this work consists of the evaluation of atmospheric pressure dielectric barrier discharges for the conversion of greenhouse gases into useful compounds. Therefore, pure CO2 feed flows are administered to the discharge zone at varying discharge frequency, power input, gas temperature and feed flow rates, aiming at the formation of CO and O-2. The discharge obtained in CO2 is characterized as a filamentary mode with a microdischarge zone in each half cycle of the applied voltage. It is shown that the most important parameter affecting the CO2- conversion levels is the gas flow rate. At low flow rates, both the conversion and the CO-yield are significantly higher. In addition, also an increase in the gas temperature and the power input give rise to higher conversion levels, although the effect on the CO-yield is limited. The optimum discharge frequency depends on the power input level and it cannot be unambiguously stated that higher frequencies give rise to increased conversion levels. A maximum CO2 conversion of 30% is achieved at a flow rate of 0.05 L min(-1), a power density of 14.75 W cm(-3) and a frequency of 60 kHz. The most energy efficient conversions are achieved at a flow rate of 0.2 L min(-1), a power density of 11 W cm(-3) and a discharge frequency of 30 kHz.
ISSN: 0963-0252
Publication status: published
KU Leuven publication type: IT
Appears in Collections:Centre for Surface Chemistry and Catalysis
× corresponding author
# (joint) last author

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